G. Passetti, C. J. Eckhardt, M. A. Sentef, and D. M. Kennes
The hybridization between light and matter forms the basis to achieve cavity control over quantum materials. In this Letter we investigate a cavity coupled to a quantum chain of interacting spinless fermions by numerically exact solutions and perturbative analytical expansions. We draw two important conclusions about such systems: (i) Specific quantum fluctuations of the matter system play a pivotal role in achieving entanglement between light and matter; and (ii) in turn, light-matter entanglement is a key ingredient to modify electronic properties by the cavity. We hypothesize that quantum fluctuations of those matter operators to which the cavity modes couple are a general prerequisite for light-matter entanglement in the ground state. Implications of our findings for light-matter-entangled phases, cavity-modified phase transitions in correlated systems, and measurement of light-matter entanglement through Kubo response functions are discussed.